All-Optical Detection of Periodic Structure of Chalcogenide Superlattice Using Coherent Folded Acoustic Phonons

Takara Suzuki, Yuta Saito, Paul Fons, Alexander V. Kolobov, Junji Tominaga, Muneaki Hase

Research output: Contribution to journalLetter

Abstract

Chalcogenide superlattices (SL) consist of alternately stacked GeTe and Sb2Te3 layers. The structure can act as a 3D topological insulator depending on the constituent layer thicknesses, making the design of the SL period a central issue for advancing chalcogenide SL as potential candidates for spin devices as well as for optimization of the current generation of phase-change memory devices. Here we explore the periodic structure of chalcogenide SL by observing coherent folded longitudinal acoustic (FLA) phonons excited by femtosecond laser pulse irradiation. The peak frequency of the FLA modes is observed to change upon variation of the thickness of the GeTe layer, which is well reproduced by means of an elastic continuum model. In addition, a new SL structure is unveiled for a sample consisting of thin GeTe and Sb2Te3 layers, which suggests intermixing of Ge atoms. This all-optical technique based on observation of coherent FLA modes offers a non-destructive characterization of superlattice structures at atomic resolution.

Original languageEnglish
Article number1800246
JournalPhysica Status Solidi - Rapid Research Letters
Volume12
Issue number9
DOIs
Publication statusPublished - 2018 Sep
Externally publishedYes

Keywords

  • acoustic phonons
  • chalcogenide superlattices
  • phase-change materials
  • ultrafast spectroscopy
  • zone-folding

ASJC Scopus subject areas

  • Materials Science(all)
  • Condensed Matter Physics

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