Measurement of Out-of-Plane Thermal Conductivity of Epitaxial YBa 2Cu 3O 7 - δ Thin Films in the Temperature Range from 10 K to 300 K by Photothermal Reflectance

Yusuke Murakami, Haruna Goto, Yoshihiro Taguchi, Yuji Nagasaka

Research output: Contribution to journalArticle

Abstract

We measured the out-of-plane (c-axis) thermal conductivity of epitaxially grown YBa 2Cu 3O 7 - δ (YBCO) thin films (250 nm, 500 nm and 1000 nm) in the temperature range from 10 K to 300 K using the photothermal reflectance technique. The technique enables us to determine the thermal conductivity perpendicular to a thin film on a substrate by curve fitting analysis of the phase lag between the thermoreflectance signal and modulated heating laser beam in the frequency range from 102Hz to 106Hz. The uncertainties of measured thermal conductivity of all samples were estimated to be within ±9% at 300 K, ±12% at 180 K, ±16% at 90 K and ±20% below 50 K. The experimental results show that the thermal conductivity is dependent on the thickness of the thin films across the entire temperature range. We also observed that the thermal conductivity of the present YBCO thin films showed T1.4 to T1.6 glass-like dependence below 50 K, even though the films are crystalline solids. In order to explain the reason for this temperature dependence, we attempted to analyze our results using phonon relaxation times for possible phonon scattering models, including stacking faults, grain boundary and tunneling states scattering models.

Original languageEnglish
Article number160
JournalInternational Journal of Thermophysics
Volume38
Issue number10
DOIs
Publication statusPublished - 2017 Oct 1

Fingerprint

thermal conductivity
reflectance
thin films
temperature
curve fitting
scattering
crystal defects
time lag
grain boundaries
relaxation time
frequency ranges
laser beams
temperature dependence
heating
glass

Keywords

  • Low temperature
  • Photothermal reflectance
  • Thermal conductivity
  • Thin film
  • YBCO

ASJC Scopus subject areas

  • Condensed Matter Physics

Cite this

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title = "Measurement of Out-of-Plane Thermal Conductivity of Epitaxial YBa 2Cu 3O 7 - δ Thin Films in the Temperature Range from 10 K to 300 K by Photothermal Reflectance",
abstract = "We measured the out-of-plane (c-axis) thermal conductivity of epitaxially grown YBa 2Cu 3O 7 - δ (YBCO) thin films (250 nm, 500 nm and 1000 nm) in the temperature range from 10 K to 300 K using the photothermal reflectance technique. The technique enables us to determine the thermal conductivity perpendicular to a thin film on a substrate by curve fitting analysis of the phase lag between the thermoreflectance signal and modulated heating laser beam in the frequency range from 102Hz to 106Hz. The uncertainties of measured thermal conductivity of all samples were estimated to be within ±9{\%} at 300 K, ±12{\%} at 180 K, ±16{\%} at 90 K and ±20{\%} below 50 K. The experimental results show that the thermal conductivity is dependent on the thickness of the thin films across the entire temperature range. We also observed that the thermal conductivity of the present YBCO thin films showed T1.4 to T1.6 glass-like dependence below 50 K, even though the films are crystalline solids. In order to explain the reason for this temperature dependence, we attempted to analyze our results using phonon relaxation times for possible phonon scattering models, including stacking faults, grain boundary and tunneling states scattering models.",
keywords = "Low temperature, Photothermal reflectance, Thermal conductivity, Thin film, YBCO",
author = "Yusuke Murakami and Haruna Goto and Yoshihiro Taguchi and Yuji Nagasaka",
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language = "English",
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T1 - Measurement of Out-of-Plane Thermal Conductivity of Epitaxial YBa 2Cu 3O 7 - δ Thin Films in the Temperature Range from 10 K to 300 K by Photothermal Reflectance

AU - Murakami, Yusuke

AU - Goto, Haruna

AU - Taguchi, Yoshihiro

AU - Nagasaka, Yuji

PY - 2017/10/1

Y1 - 2017/10/1

N2 - We measured the out-of-plane (c-axis) thermal conductivity of epitaxially grown YBa 2Cu 3O 7 - δ (YBCO) thin films (250 nm, 500 nm and 1000 nm) in the temperature range from 10 K to 300 K using the photothermal reflectance technique. The technique enables us to determine the thermal conductivity perpendicular to a thin film on a substrate by curve fitting analysis of the phase lag between the thermoreflectance signal and modulated heating laser beam in the frequency range from 102Hz to 106Hz. The uncertainties of measured thermal conductivity of all samples were estimated to be within ±9% at 300 K, ±12% at 180 K, ±16% at 90 K and ±20% below 50 K. The experimental results show that the thermal conductivity is dependent on the thickness of the thin films across the entire temperature range. We also observed that the thermal conductivity of the present YBCO thin films showed T1.4 to T1.6 glass-like dependence below 50 K, even though the films are crystalline solids. In order to explain the reason for this temperature dependence, we attempted to analyze our results using phonon relaxation times for possible phonon scattering models, including stacking faults, grain boundary and tunneling states scattering models.

AB - We measured the out-of-plane (c-axis) thermal conductivity of epitaxially grown YBa 2Cu 3O 7 - δ (YBCO) thin films (250 nm, 500 nm and 1000 nm) in the temperature range from 10 K to 300 K using the photothermal reflectance technique. The technique enables us to determine the thermal conductivity perpendicular to a thin film on a substrate by curve fitting analysis of the phase lag between the thermoreflectance signal and modulated heating laser beam in the frequency range from 102Hz to 106Hz. The uncertainties of measured thermal conductivity of all samples were estimated to be within ±9% at 300 K, ±12% at 180 K, ±16% at 90 K and ±20% below 50 K. The experimental results show that the thermal conductivity is dependent on the thickness of the thin films across the entire temperature range. We also observed that the thermal conductivity of the present YBCO thin films showed T1.4 to T1.6 glass-like dependence below 50 K, even though the films are crystalline solids. In order to explain the reason for this temperature dependence, we attempted to analyze our results using phonon relaxation times for possible phonon scattering models, including stacking faults, grain boundary and tunneling states scattering models.

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