Non-Markovian effects of intermolecular vibrational coherence on femtosecond time-resolved coherent anti-Stokes Raman scattering from molecules in condensed phases

M. Sugawara, M. Hayashi, Y. Fujimura

Research output: Contribution to journalArticle

Abstract

Non-Markovian effects of intermolecular vibrational coherences on femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) from a molecular mixture are theoretically studied. The non-Markovian behavior of intermolecular vibrational coherence transfers based on a stochastic model results in the suppresion of the frequency shifts of quantum beats in the time-resolved CARS profiles compared with the case in the Markovian approximation.

Original languageEnglish
Pages (from-to)346-352
Number of pages7
JournalChemical Physics Letters
Volume189
Issue number4-5
DOIs
Publication statusPublished - 1992 Feb 14

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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