Suppression of intramolecular vibrational energy redistribution by intense CW-laser fields

M. Sugawara

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Abstract

We present a quantum control scheme which realizes suppression of the intramolecular vibrational energy redistribution (IVR). In this scheme, we utilize effective decomposition brought by intense CW-laser fields, which enables to exclude the doorway state coupled to background manifolds. In doing so, we introduce a helper state and make it optically coupled with the doorway state through the intense CW-laser field. We have applied the present scheme to both the Bixon-Jortner model and the SCCl2 model system.

Original languageEnglish
Article number584082
JournalAdvances in Physical Chemistry
Volume2011
DOIs
Publication statusPublished - 2011 Sep 16

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ASJC Scopus subject areas

  • Physical and Theoretical Chemistry

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