Third-order optical nonlinearity due to excitons and biexcitons in a self-organized quantum-well material (C6H13NH3)2PbI4

J. Ishi, M. Mizuno, H. Kunugita, K. Ema, S. Iwamoto, S. Hayase, T. Kondo, R. Ito

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Abstract

Third-order optical nonlinearity around the exciton resonance in (C6H13NH3)2PbI4 was measured using time-integrated and spectrally-resolved four-wave-mixing (FWM) techniques. For excitation below the exciton resonance, biexciton contribution to the FWM signals was observed. The dephasing energy of the biexcitons was estimated to be larger than 10 meV.

Original languageEnglish
Pages (from-to)153-159
Number of pages7
JournalJournal of Nonlinear Optical Physics and Materials
Volume7
Issue number1
DOIs
Publication statusPublished - 1998 Mar

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ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Atomic and Molecular Physics, and Optics
  • Physics and Astronomy (miscellaneous)

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