Imaging and Characterizing Long-Range Surface Plasmon Polaritons Propagating in a Submillimeter Scale by Two-Color Two-Photon Photoelectron Emission Microscopy

Masahiro Shibuta, Toyoaki Eguchi, Atsushi Nakajima

研究成果: Article

9 引用 (Scopus)

抄録

Long-range surface plasmon polaritons (SPPs), which propagate along metal/dielectric interfaces to submillimeter distances in the range of near-infrared (NIR) excitation wavelength, were examined by two-color two-photon photoelectron emission microscopy (2P-PEEM). Interferences between incident NIR photons and SPPs excited by the NIR photons at surface defects were imaged by detecting photoelectrons emitted from a gold surface, assisted by simultaneously irradiated ultraviolet photons which are to overcome the workfunction of the surface. The wavelength of the interference beat depends sensitively on the NIR wavelength. By analyzing the interference beat, the dispersion curve as well as phase and group velocities of SPP's were experimentally obtained. The results closely match the theoretical one based on the Drude free electron model, indicating that two-color 2P-PEEM is applicable not only to the visualization of NIR-excited SPPs but also to the quantitative analysis of its physical properties. This method will be widely used to observe SPPs for various artificial plasmonic devices.

元の言語English
ページ(範囲)1411-1415
ページ数5
ジャーナルPlasmonics
8
発行部数3
DOI
出版物ステータスPublished - 2013 9

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Photoelectrons
Photons
Microscopy
Microscopic examination
Color
Imaging techniques
Infrared radiation
Wave interference
Wavelength
Gold
Metals
Surface defects
Electrons
Equipment and Supplies
Visualization
Physical properties
Chemical analysis

ASJC Scopus subject areas

  • Biochemistry
  • Biophysics
  • Biotechnology

これを引用

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title = "Imaging and Characterizing Long-Range Surface Plasmon Polaritons Propagating in a Submillimeter Scale by Two-Color Two-Photon Photoelectron Emission Microscopy",
abstract = "Long-range surface plasmon polaritons (SPPs), which propagate along metal/dielectric interfaces to submillimeter distances in the range of near-infrared (NIR) excitation wavelength, were examined by two-color two-photon photoelectron emission microscopy (2P-PEEM). Interferences between incident NIR photons and SPPs excited by the NIR photons at surface defects were imaged by detecting photoelectrons emitted from a gold surface, assisted by simultaneously irradiated ultraviolet photons which are to overcome the workfunction of the surface. The wavelength of the interference beat depends sensitively on the NIR wavelength. By analyzing the interference beat, the dispersion curve as well as phase and group velocities of SPP's were experimentally obtained. The results closely match the theoretical one based on the Drude free electron model, indicating that two-color 2P-PEEM is applicable not only to the visualization of NIR-excited SPPs but also to the quantitative analysis of its physical properties. This method will be widely used to observe SPPs for various artificial plasmonic devices.",
keywords = "Interference beat, Photoelectron emission microscope, Surface plasmon polaritons, Two-photon photoemission",
author = "Masahiro Shibuta and Toyoaki Eguchi and Atsushi Nakajima",
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T1 - Imaging and Characterizing Long-Range Surface Plasmon Polaritons Propagating in a Submillimeter Scale by Two-Color Two-Photon Photoelectron Emission Microscopy

AU - Shibuta, Masahiro

AU - Eguchi, Toyoaki

AU - Nakajima, Atsushi

PY - 2013/9

Y1 - 2013/9

N2 - Long-range surface plasmon polaritons (SPPs), which propagate along metal/dielectric interfaces to submillimeter distances in the range of near-infrared (NIR) excitation wavelength, were examined by two-color two-photon photoelectron emission microscopy (2P-PEEM). Interferences between incident NIR photons and SPPs excited by the NIR photons at surface defects were imaged by detecting photoelectrons emitted from a gold surface, assisted by simultaneously irradiated ultraviolet photons which are to overcome the workfunction of the surface. The wavelength of the interference beat depends sensitively on the NIR wavelength. By analyzing the interference beat, the dispersion curve as well as phase and group velocities of SPP's were experimentally obtained. The results closely match the theoretical one based on the Drude free electron model, indicating that two-color 2P-PEEM is applicable not only to the visualization of NIR-excited SPPs but also to the quantitative analysis of its physical properties. This method will be widely used to observe SPPs for various artificial plasmonic devices.

AB - Long-range surface plasmon polaritons (SPPs), which propagate along metal/dielectric interfaces to submillimeter distances in the range of near-infrared (NIR) excitation wavelength, were examined by two-color two-photon photoelectron emission microscopy (2P-PEEM). Interferences between incident NIR photons and SPPs excited by the NIR photons at surface defects were imaged by detecting photoelectrons emitted from a gold surface, assisted by simultaneously irradiated ultraviolet photons which are to overcome the workfunction of the surface. The wavelength of the interference beat depends sensitively on the NIR wavelength. By analyzing the interference beat, the dispersion curve as well as phase and group velocities of SPP's were experimentally obtained. The results closely match the theoretical one based on the Drude free electron model, indicating that two-color 2P-PEEM is applicable not only to the visualization of NIR-excited SPPs but also to the quantitative analysis of its physical properties. This method will be widely used to observe SPPs for various artificial plasmonic devices.

KW - Interference beat

KW - Photoelectron emission microscope

KW - Surface plasmon polaritons

KW - Two-photon photoemission

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